DC Field | Value | Language |
---|---|---|
dc.contributor.author | CHOI, SUNGHO | - |
dc.contributor.author | Bin Wang | - |
dc.contributor.author | Jaegeon Ryu | - |
dc.contributor.author | Gyujin Song | - |
dc.contributor.author | Dongki Hong | - |
dc.contributor.author | Chihyun Hwang | - |
dc.contributor.author | Xiong Chen | - |
dc.contributor.author | Bo Wang | - |
dc.contributor.author | Wei Li | - |
dc.contributor.author | Hyun-Kon Song | - |
dc.contributor.author | Soojin Park | - |
dc.contributor.author | Rodney S. Ruoff | - |
dc.date.accessioned | 2020-10-06T04:50:15Z | - |
dc.date.available | 2020-10-06T04:50:15Z | - |
dc.date.created | 2020-08-20 | - |
dc.date.issued | 2018-02 | - |
dc.identifier.issn | 1936-0851 | - |
dc.identifier.uri | https://oasis.postech.ac.kr/handle/2014.oak/104251 | - |
dc.description.abstract | We show that a high energy density can be achieved in a practical manner with freestanding electrodes without using conductive carbon, binders, and current collectors. We made and used a folded graphene composite electrode designed for a high areal capacity anode. The traditional thick graphene composite electrode, such as made by filtering graphene oxide to create a thin film and reducing it such as through chemical or thermal methods, has sluggish reaction kinetics. Instead, we have made and tested a thin composite film electrode that was folded several times using a water-assisted method; it provides a continuous electron transport path in the fold regions and introduces more channels between the folded layers, which significantly enhances the electron/ion transport kinetics. A fold electrode consisting of SnO2/graphene with high areal loading of 5 mg cm(-2) has a high areal capacity of 4.15 mAh cm(-2), well above commercial graphite anodes (2.50-3.50 mAh cm(-2)), while the thickness is maintained as low as 20 pm. The fold electrode shows stable cycling over 500 cycles at 1.70 mA cm(-2) and improved rate capability compared to thick electrodes with the same mass loading but without folds. A electrode coupled with LiCoO2 cathode was assembled and delivered an areal capacity of 2.84 mAh cm(-2) after 300 cycles. This folding strategy can be extended to other electrode materials and rechargeable batteries. | - |
dc.language | English | - |
dc.publisher | American Chemical Society | - |
dc.relation.isPartOf | ACS Nano | - |
dc.title | Folding Graphene Film Yields High Areal Energy Storage in Lithium-Ion Batteries | - |
dc.type | Article | - |
dc.identifier.doi | 10.1021/acsnano.7b08489 | - |
dc.type.rims | ART | - |
dc.identifier.bibliographicCitation | ACS Nano, v.12, no.2, pp.1739 - 1746 | - |
dc.identifier.wosid | 000426615600085 | - |
dc.citation.endPage | 1746 | - |
dc.citation.number | 2 | - |
dc.citation.startPage | 1739 | - |
dc.citation.title | ACS Nano | - |
dc.citation.volume | 12 | - |
dc.contributor.affiliatedAuthor | CHOI, SUNGHO | - |
dc.identifier.scopusid | 2-s2.0-85042692621 | - |
dc.description.journalClass | 1 | - |
dc.description.journalClass | 1 | - |
dc.description.isOpenAccess | N | - |
dc.type.docType | Article | - |
dc.subject.keywordPlus | FREE ANODE | - |
dc.subject.keywordPlus | CAPACITY | - |
dc.subject.keywordPlus | PAPER | - |
dc.subject.keywordPlus | OXIDE | - |
dc.subject.keywordPlus | NANOCOMPOSITES | - |
dc.subject.keywordPlus | PERFORMANCE | - |
dc.subject.keywordPlus | ELECTRODES | - |
dc.subject.keywordPlus | STABILITY | - |
dc.subject.keywordPlus | COMPOSITE | - |
dc.subject.keywordPlus | AEROGELS | - |
dc.subject.keywordAuthor | folding | - |
dc.subject.keywordAuthor | graphene composite films | - |
dc.subject.keywordAuthor | high mass loading | - |
dc.subject.keywordAuthor | high areal capacity | - |
dc.subject.keywordAuthor | lithium-ion batteries | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical | - |
dc.relation.journalWebOfScienceCategory | Nanoscience & Nanotechnology | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalResearchArea | Science & Technology - Other Topics | - |
dc.relation.journalResearchArea | Materials Science | - |
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