DC Field | Value | Language |
---|---|---|
dc.contributor.author | Cheol-Joo Kim | - |
dc.contributor.author | A. Sánchez-Castillo | - |
dc.contributor.author | Zack Ziegler | - |
dc.contributor.author | Yui Ogawa | - |
dc.contributor.author | Cecilia Noguez | - |
dc.contributor.author | Jiwoong Park | - |
dc.date.accessioned | 2019-04-07T19:59:55Z | - |
dc.date.available | 2019-04-07T19:59:55Z | - |
dc.date.created | 2019-03-15 | - |
dc.date.issued | 2016-06 | - |
dc.identifier.issn | 1748-3387 | - |
dc.identifier.uri | https://oasis.postech.ac.kr/handle/2014.oak/96314 | - |
dc.description.abstract | Chiral materials possess left- and right-handed counterparts linked by mirror symmetry. These materials are useful for advanced applications in polarization optics(1,2), stereochemistry(3,4) and spintronics(5,6). In particular, the realization of spatially uniform chiral films with atomic-scale control of their handedness could provide a powerful means for developing nanodevices with novel chiral properties. However, previous approaches based on natural or grown films(1,2,7,8), or arrays of fabricated building blocks(9-11), could not offer a direct means to program intrinsic chiral properties of the film on the atomic scale. Here, we report a chiral stacking approach, where two-dimensional materials are positioned layer-by-layer with precise control of the interlayer rotation (theta) and polarity, resulting in tunable chiral properties of the final stack. Using this method, we produce left-and right-handed bilayer graphene, that is, a two-atom-thick chiral film. The film displays one of the highest intrinsic ellipticity values (6.5 deg mu m(-1)) ever reported, and a remarkably strong circular dichroism (CD) with the peak energy and sign tuned by. and polarity. We show that these chiral properties originate from the large in-plane magnetic moment associated with the interlayer optical transition. Furthermore, we show that we can program the chiral properties of atomically thin films layer-by-layer by producing three-layer graphene films with structurally controlled CD spectra. | - |
dc.language | English | - |
dc.publisher | NATURE PUBLISHING GROUP | - |
dc.relation.isPartOf | Nature Nanotechnology | - |
dc.title | Chiral atomically thin films | - |
dc.type | Article | - |
dc.identifier.doi | 10.1038/NNANO.2016.3 | - |
dc.type.rims | ART | - |
dc.identifier.bibliographicCitation | Nature Nanotechnology, v.11, no.6, pp.520 - + | - |
dc.identifier.wosid | 000377476800010 | - |
dc.citation.endPage | + | - |
dc.citation.number | 6 | - |
dc.citation.startPage | 520 | - |
dc.citation.title | Nature Nanotechnology | - |
dc.citation.volume | 11 | - |
dc.contributor.affiliatedAuthor | Cheol-Joo Kim | - |
dc.identifier.scopusid | 2-s2.0-84959120884 | - |
dc.description.journalClass | 1 | - |
dc.description.journalClass | 1 | - |
dc.description.isOpenAccess | N | - |
dc.type.docType | Article | - |
dc.subject.keywordPlus | WALLED CARBON NANOTUBES | - |
dc.subject.keywordPlus | VAN-HOVE SINGULARITIES | - |
dc.subject.keywordPlus | CIRCULAR-DICHROISM | - |
dc.subject.keywordPlus | GRAPHENE | - |
dc.subject.keywordPlus | HETEROSTRUCTURES | - |
dc.subject.keywordPlus | SPIN | - |
dc.relation.journalWebOfScienceCategory | Nanoscience & Nanotechnology | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
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